2980. p,p′-Diaminodiphenylmethane

Nomenclature

CAS number: 101-77-9
4,4′-Methylenebis[benzenamine]; 4,4′-methylenedianiline.
C13H14N2; mol wt 198.26.
C 78.75%, H 7.12%, N 14.13%.

Description and references

Prepn from aniline and formaldehyde: Scanlon, J. Am. Chem. Soc. 57, 887 (1935); by hydrogenolysis of p,p′-diaminobenzophenone with LiAlH4: Conover, Tarbell, ibid. 72, 3586 (1950). Identified as causative agent in clinical outbreak of hepatoxicity called Epping Jaundice: H. Kopelman et al., Br. Med. J. 1, 514 (1966); D. B. McGill, J. D. Motto, N. Engl. J. Med. 291, 278 (1974). Review of toxicology and human exposure: Toxicological Profile for Methylenedianiline (PB99-102568, 1998) 194 pp.

Chemical structure

Properties

Crystals from water or benzene. mp 91.5-92°. bp768 398-399°; bp18 257°; bp15 249-253°; bp9 232°. Slightly sol in cold water. Very sol in alcohol, benzene, ether.

Caution

Potential symptoms of overexposure by ingestion are jaundice, weakness, abdominal pain, nausea, vomiting, anorexia, fever, chills, hepatotoxicity (Kopelman). Direct contact may cause skin irritation (PB99-102568). This substance and its dihydrochloride are reasonably anticipated to be human carcinogens: Report on Carcinogens, Eleventh Edition (PB2005-104914, 2004) p III-169.

Use

As chemical intermediate in prodn of isocyanates and polyisocyantes for prepn of polyurethane foams, Spandex fibers; as curing agent for epoxy resins and urethane elastomers; in production of polyamides; in the determination of tungsten and sulfates; in prepn of azo dyes; as corrosion inhibitor.