5522. Lithium Amide

Nomenclature

CAS number: 7782-89-0
Lithamide.
H2LiN; mol wt 22.96.
H 8.78%, Li 30.23%, N 61.00%.
LiNH2.

Description and references

Prepd from Li + NH3: Titherley, J. Chem. Soc. 65, 517 (1894); Ruff, Geisel Ber. 39, 840 (1906); 44, 505 (1911); Campbell et al., Proc. Indiana Acad. Sci. 50, 123 (1940); Schenk in Handbook of Preparative Inorganic Chemistry vol. 1, G. Brauer, Ed. (Academic Press, New York, 2nd ed., 1963) p 463. See also Inorg. Synth. 2, 135. Crystal structure: Juza, Opp, Z. Anorg. Allg. Chem. 266, 313 (1951).

Properties

Tetragonal crystal structure, d 1.18. mp 380-400°. Sublimes in NH3 current. When heated in vacuo to 450°, NH3 is given off and Li2NH forms, which dec ≈750-800°. Heat of formation: 42 kcal/mole at 18° and 760 mm Hg. Stable in air-tight containers at room temp. Dec by water to form LiOH + NH3, slowly when in lumps, faster as the particle size decreases. Insol in anhydr ether, benzene, toluene.

Use

In Claisen condensations, alkylation of nitriles and ketones, synthesis of ethynyl compds, acetylenic carbinols.