10173. Zirconium

Nomenclature

CAS number: 7440-67-7

Description and references

Zr; at. wt 91.224; at. no. 40; valence 4; also 3. Group IVB (4). Five naturally occurring isotopes: 90 (51.46%); 91 (11.23%); 92 (17.11%); 94 (17.40%); 96 (2.80%); artificial radioactive isotopes: 81-89, 93, 95, 97-99. Occurrence in earth's crust: 0.023%. Occurs in the minerals zircon, malacon, baddeleyite, zirkelite, eudialyte; frequently found in the rare-earth minerals; in monazite sand. Discovered by Klaproth in 1789; prepd by Berzelius in 1824. Prepn: Fast, Z. Anorg. Chem. 239, 145 (1938); purification of zirconium by ion exchange columns: Ayres, J. Am. Chem. Soc. 69, 1879 (1947). Sepn of zirconium and hafnium: Fischer et al., Angew. Chem. Int. Ed. 5, 15 (1966). Reviews of zirconium and its compds: W. B. Blumenthal, The Chemical Behavior of Zirconium (Van Nostrand, Princeton, 1958); Gmelins, Zirconium (8th ed.) 42, (1958) 448 pp; Larsen, “Zirconium and Hafnium Chemistry” in Adv. Inorg. Chem. Radiochem. 13, 1-333 (1970); Bradley, Thornton, “Zirconium and Hafnium” in Comprehensive Inorganic Chemistry vol. 3, J. C. Bailar, Jr. et al., Eds. (Pergamon Press, Oxford, 1973) pp 419-490.

Properties

Bluish-black, amorphous powder or grayish-white lustrous metal (platelets or flakes) of hexagonal lattice below 865°, body-centered cubic above 865°, mp 1857°; bp 3577°. d 6.5. Brinnell hardness: 85. Can absorb up to 10 atoms per cent of oxygen or nitrogen. Flammable; spontaneously combustible. Reacts with hydrofluoric acid, aqua regia, hot phosphoric acid. Not attacked by cold, very slightly attacked by hot, concd sulfuric or hydrochloric acid; not attacked by nitric acid. Attacked by fused potassium hydroxide or nitrate. On prolonged heating the compact form combines with oxygen, nitrogen, carbon, and the halogens. The powder form has a very low ignition temp and is very explosive when mixed with oxidizing agents.

Caution

Zirconium and its salts generally have low systemic toxicity. A granulomatous disease of the skin, particularly in the axilla, has been reported in users of a deodorant contg sodium zirconium lactate: see E. Browning, Toxicity of Industrial Metals (Appleton-Century-Crofts, New York, 2nd ed., 1969) pp 356-360. Consult latest Government regulations on use in aerosol antiperspirants.

Use

Pure zirconium (hafnium-free) is a valuable structural material for atomic reactors because of its low nuclear cross-section and high corrosion and heat resistance. Because of hafnium's high neutron absorption characteristics, it must be removed from zirconium which is to be used in nuclear reactors; removal unnecessary for other commercial purposes. As an ingredient of priming or explosive mixtures; flashlight powders; as deoxidizer in metallurgy; as “getter” in vacuum tubes; in constructing rayon spinnerets in lamp filaments, flash bulbs.