Description and references
Antibiotic complex composed of neomycins A,
B and C. Produced by Streptomyces fradiae: Waksman, Lechevalier, Science 109, 305 (1949); Waksman et al., J. Clin. Invest. 28, 934 (1949); Swart et al., ibid. 1045; Waksman, Lechevalier, US 2799620 (1957). Purification: Jackson, US 2848365 (1958 to Upjohn); Haak, US 3108996 (1963 to Upjohn). Recovery: Miller, US 3005815 (1961 to Merck & Co.); Moses, US 3022228 (1962 to Penick); GB 945475 (1964 to O.W.G. Chemie). Characterization:
Peck et al., J. Am. Chem. Soc. 71, 2590 (1949); Regna, Murphy, ibid. 72, 1045 (1950); Dutcher et al., ibid. 73, 1384 (1951).
Structure of neomycins B and C: K. L. Rinehart et al., ibid. 79, 4567, 4568
(1957); ibid. 84, 3216,
3218 (1962). Abs config of neomycin C: M. Hichens, K. L. Rinehart, ibid. 85, 1547 (1963). Total
synthesis of neomycin C: S. Umewaza, Y. Nishimura, J. Antibiot. 30, 189 (1977); S.
Umewaza et al., Bull. Chem. Soc.
Jpn. 53, 3259 (1980); of neomycin B: T. Usui,
S. Umezawa, J. Antibiot. 40, 1464 (1987). Monographs: S. A. Waksman, Neomycin (Rutgers Univ. Press, New Brunswick,
N. J., 1953) 219 pp; K. L. Rinehart, Jr., The Neomycins and Related Antibiotics (Wiley, New York,
1964) 137 pp. Comprehensive description: W. F. Heyes, Anal. Profiles Drug Subs. 8, 399-488
(1979).
Derivative
Neomycin B.
Nomenclature
CAS number: 119-04-0
Antibiotique EF 185; framycetin; Enterfram; Framygen; Actilin.
C
23H
46N
6O
13; mol wt 614.64.
C 44.94%, H 7.54%, N 13.67%, O 33.84%.
Properties
Identity of neomycin B and framycetin: K. L.
Rinehart et al., ibid. 82, 3938 (1960). Yields on hydrolysis neamine and neobiosamine B. Structure of neobiosamine B: K. L. Rinehart et
al., J. Am. Chem. Soc. 82, 2970 (1960).Derivative
Neomycin B hydrochloride.
Nomenclature
CAS number: 25389-99-5
Properties
Amorphous white powder. [α]D20 +57° (H2O). Soly in mg/ml at ≈28°: water 15.0; methanol 5.7; ethanol
0.65; isopropanol 0.05; isoamyl alcohol 0.33; cyclohexane 0.06; benzene
0.03. Practically insol in acetone, ether, other organic solvents.
For additional soly data see Weiss et al., Antibiot. Chemother. 7, 374 (1957).Derivative
Neomycin B sulfate.
Nomenclature
CAS number: 1405-10-3
Biosol (Biokema); Bykomycin (Byk Gulden); Endomixin (Lusofarmaco); Fraquinol; Myacine; Neosulf; Neomix (Tuco); Neobrettin (Norbrook); Nivemycin (Boots); Soframycin (HMR); Tuttomycin.
Properties
Amorphous white powder. Practically tasteless.
[α]D20 +54° (c = 2 in H2O). Soly in mg/ml at ≈28°:
water 6.3; methanol 0.225; ethanol 0.095; isopropanol 0.082; isoamyl
alcohol, 0.247; cyclohexane 0.08; benzene 0.05. Practically insol
in acetone, ether, chloroform. Aq solns are fairly stable at pH 2
to 9. Highly purified prepns are very stable to alkali and unstable
to acids. Refluxing with barium hydroxide for 18 hrs showed no loss
of activity. Boiling with mineral acids yields an aldehyde, characterized
as furfural, and an organic base.Derivative
Neomycin C.
Nomenclature
CAS number: 66-86-4
C
23H
46N
6O
13; mol wt 614.64.
C 44.94%, H 7.54%, N 13.67%, O 33.84%.
Properties
Yields on hydrolysis neamine and neobiosamine C. Structure of neobiosamine C: K. L. Rinehart, P. Woo, J. Am. Chem. Soc. 80, 6463 (1958).Antibacterial.
Antibacterial.