8347. Samarium

Nomenclature

CAS number: 7440-19-9

Description and references

Sm; at. wt 150.36; at. no. 62; valences 2, 3. A lanthanide belonging to the cerium group of rare earth metals; named for the mineral “samarskite” from which it was isolated. Naturally occurring isotopes (mass numbers): 144 (3.1%); 147 (15.0%), radioactive, T 1/2 1.06 × 1011 years, α-emitter; 148 (11.3%), radioactive, T 1/2 7 × 1015 years, α-emitter; 149 (13.8%); 150 (7.4%); 152 (26.7%); 154 (22.7%). Known artificial radioactive isotopes: 133-143; 145; 146; 151; 153; 155-158. Abundance in earth's crust: 6.47-7.0 ppm. Commercially important sources are the rare earth minerals monazite and bastnaesite; also occurs in samarskite, cerite, orthite, ytterbite, and fluorspar. Isoln: L. de Boisbaudran, Compt. Rend. 88, 322 (1879); 89, 212 (1880). Sepn by crystn of the nitrates: Demarcay, ibid. 122, 728 (1896); Feit, Przibylla, Z. Anorg. Chem. 43, 203 (1905). Sepn of metal: Schumacher, Harris, J. Am. Chem. Soc. 48, 3108 (1926); by reduction of salts: Marsh, J. Chem. Soc. 1942, 398, 523; 1943, 8; Daane et al., J. Am. Chem. Soc. 75, 2272 (1953); Onstott, ibid. 75, 5128 (1953); 77, 812 (1955). Toxicity study: Haley, J. Pharm. Sci. 54, 663 (1965). Reviews of prepn, properties and compds: Prandtl, Z. Anorg. Allg. Chem. 238, 321-334 (1938); The Rare Earths, F. H. Spedding, A. H. Daane (Krieger, Huntington, N.Y., 1971, reprint of 1961 ed) 641 pp; Hulet, Bode, “Separation Chemistry of the Lanthanides and Transplutonium Actinides” in MTP Int. Rev. Sci.: Inorg. Chem., Ser. One Vol. 7, K. W. Bagnall, Ed. (University Park Press, Baltimore, 1972) pp 1-45; Moeller, “The Lanthanides” in Comprehensive Inorganic Chemistry Vol. 4, J. C. Bailar Jr. et al., Eds. (Pergamon Press, Oxford, 1973) pp 1-101; F. H. Spedding in Kirk-Othmer Encyclopedia of Chemical Technology vol. 19, (John Wiley & Sons, New York, 3rd ed., 1982) pp 833-854; Chemistry of the Elements, N. N. Greenwood, A. Earnshaw, Eds. (Pergamon Press, New York, 1984) pp 1423-1449. Brief review of properties: G. T. Seaborg, Radiochim. Acta 61, 115-122 (1993).

Properties

Yellow metal; tarnishes on exposure to air. Hardest metal of the cerium group. Crystalline forms: rhombohedral α-form, d 7.536, transforms to β-form at 917°; body-centered cubic β-form exists at >917°. mp 1074°. bp 1794°. Heat of fusion: 8.623 kJ/mol. Heat of sublimation (25°): 206.7 kJ/mol. E°(aq) Sm3+/Sm -2.41 V (calc).

Derivative

Oxide.
Sm2O3; mol wt 348.72.
Sm 86.24%, O 13.76%.

Properties

Yellowish-white powder. d 8.347.

Derivative

Hydroxide.
Sm(OH)3; mol wt 201.38.
Sm 74.66%, O 23.83%, H 1.50%.

Properties

Gelatinous precipitate.

Derivative

Trichloride.
SmCl3; mol wt 256.72.
Sm 58.57%, Cl 41.43%.

Properties

White-yellowish powder. d 4.465, mp 686°. Forms addition compds with ammonia. Forms a hexahydrate, SmCl3.6H2O, d 2.382, yellow crystalline plates. By reducing the anhydr trichloride at high temps with hydrogen, ammonia or aluminum powder, samarium dichloride is obtained. LD50 in mice (mg/kg): 585 i.p.; >2000 orally (Haley).

Derivative

Dichloride.
SmCl2; mol wt 221.27.
Sm 67.95%, Cl 32.05%.

Properties

Dark brown crystalline mass. d22 3.687. Practically insol in alcohol. Dec by water.

Derivative

Sulfate.
Sm2(SO4)3; mol wt 588.91.
Sm 51.06%, S 16.33%, O 32.60%.

Properties

Octahydrate, light yellow crystals, d18 2.930. Sparingly sol in water.

Use

Oxide in control rods of some commercial nuclear power reactors. Alloys with cobalt to produce extremely stong permanent magnets.